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A sensitivity study for far infrared balloon-borne limb emission sounding of stratospheric trace gases

机译:平流层痕量气体的远红外气球载肢发射探测灵敏度研究

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摘要

This paper presents a sensitivity study performed for trace gases retrieval from synthetic observations by TELIS (TErahertz and submillimeter LImb Sounder) which is a stratospheric balloon-borne cryogenic heterodyne spectrometer. Issues pertaining to hydroxyl radical (OH) retrieval from the far infrared measurements by the 1.8 THz channel are addressed. The study is conducted by a retrieval code PILS (Profile Inversion for Limb Sounding) developed to solve the nonlinear inverse problems arising in the analysis of infrared/microwave limb sounding measurements. PILS combines a line-by-line forward model with automatic differentiation for computing Jacobians and employs regularized nonlinear least squares inversion. We examine the application of direct and iterative regularization methods and evaluate the performance of single- and multi-profile retrievals. Sensitivities to expected errors in calibration procedure, instrumental knowledge and atmospheric profiles have been analyzed. Nonlinearity effect, inaccurate sideband ratio, and pointing error turned out to be the dominant error sources. Furthermore, the capability of multi-channel simultaneous retrieval from the far infrared and submillimeter data has been investigated. The errors and averaging kernels infer that the quality of the obtained hydrogen chloride (HCl) can be improved by significantly better exploitation of information from the observations.
机译:本文介绍了由TELIS(TErahertz和亚毫米LImb Sounder)进行的合成观测所进行的痕量气体检索的灵敏度研究,这是一个平流层气球式低温外差光谱仪。解决了与通过1.8 THz通道从远红外测量中检索到的羟基自由基(OH)有关的问题。这项研究由检索代码PILS(肢体测深剖面反转)进行,旨在解决在红外/微波肢体测深分析中出现的非线性逆问题。 PILS将逐行正向模型与自动微分相结合以计算Jacobian,并采用正则化的非线性最小二乘反演。我们研究了直接和迭代正则化方法的应用,并评估了单配置文件检索和多配置文件检索的性能。分析了对校准程序,仪器知识和大气剖面中预期误差的敏感性。非线性效应,不正确的边带比率和指向误差被证明是主要的误差源。此外,还研究了从远红外和亚毫米波数据进行多通道同时检索的能力。误差和平均内核推断,可以通过显着更好地利用来自观测的信息来提高获得的氯化氢(HCl)的质量。

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